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Modelling and identification of the dominant phenomena in hydrogen fuel-cells by the application of DRT analysis

dc.contributor.authorLopes, Vitor V.
dc.contributor.authorRangel, C. M.
dc.contributor.authorNovais, Augusto Q.
dc.date.accessioned2014-02-13T12:08:16Z
dc.date.available2014-02-13T12:08:16Z
dc.date.issued2013
dc.description.abstractThis paper proposes the use of the distribution of relaxation times (DRT) for the analysis of the dynamic behavior of hydrogen fuel-cells. With this aim it presents a new method to compute the DRT directly from electrochemical impedance spectroscopy (EIS) data. The method is formulated as a nonconvex complex domain optimization problem where each EIS spectra is approximated by a general fractional-order Legendre basis. The DRT is computed directly from the Legendre basis functions and validated against the experimental data. The method is tested with real EIS data collected from an hydrogen polymer electrolyte fuel-cell under different operating conditions and the results are discussed.por
dc.identifier.citationLopes, Vitor V.; Rangel, Carmen M.; Novais, Augusto Q. Modelling and identification of the dominant phenomena in hydrogen fuel-cells by the application of DRT analysis. In: Computer Aided Chemical Engineering, 2013, Vol. 32, p. 283-288por
dc.identifier.urihttp://hdl.handle.net/10400.9/2192
dc.language.isoengpor
dc.publisherElsevierpor
dc.relation.publisherversionhttp://dx.doi.org/10.1016/B978-0-444-63234-0.50048-8por
dc.subjectHydrogen fuel-cellspor
dc.subjectImpedance spectroscopypor
dc.subjectDistribution relaxation timespor
dc.titleModelling and identification of the dominant phenomena in hydrogen fuel-cells by the application of DRT analysispor
dc.typejournal article
dspace.entity.typePublication
oaire.citation.endPage288por
oaire.citation.startPage283por
oaire.citation.titleComputer Aided Chemical Engineeringpor
oaire.citation.volume32por
person.familyNameRangel
person.givenNameCarmen M.
person.identifier.ciencia-idAA13-FF7C-9E29
person.identifier.orcid0000-0001-7996-8142
person.identifier.ridD-5477-2011
person.identifier.scopus-author-id7006108156
rcaap.rightsopenAccesspor
rcaap.typearticlepor
relation.isAuthorOfPublication804e595a-d539-46a2-ae78-6cadc8ca9457
relation.isAuthorOfPublication.latestForDiscovery804e595a-d539-46a2-ae78-6cadc8ca9457

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